Reaction dynamics of NO2 decomposition on Ge: An example of dissociative desorption

A. Mödl; H. Robota; J. Segner; W. Vielhaber; Ming-Chang Lin; G. Ertl

doi:10.1016/0039-6028(86)90604-7

Reaction dynamics of NO₂ decomposition on Ge: An example of dissociative desorption

A. Mödl^*, H. Robota, J. Segner, W. Vielhaber, Ming-Chang Lin, G. Ertl

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摘要

The reaction NO₂ → NO + O_ad at aGe surface was studied by combined molecular beam and laser-induced fluorescence (LIF) techniques. The rotational state distribution of the NO formed is non-Boltzmann, in contrast to NO molecules undergoing trapping/desorption. It is concluded that NO formed by NO₂ decomposition is directly released into the gas phase (dissociative desorption) without being intermediately thermally accommodated to the surface.

原文	English
期刊	Surface Science
卷	169
發行號	2-3
DOIs	https://doi.org/10.1016/0039-6028(86)90604-7
出版狀態	Published - 2 4月 1986

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10.1016/0039-6028(86)90604-7

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abstract = "The reaction NO2 → NO + Oad at aGe surface was studied by combined molecular beam and laser-induced fluorescence (LIF) techniques. The rotational state distribution of the NO formed is non-Boltzmann, in contrast to NO molecules undergoing trapping/desorption. It is concluded that NO formed by NO2 decomposition is directly released into the gas phase (dissociative desorption) without being intermediately thermally accommodated to the surface.",

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T2 - An example of dissociative desorption

AU - Mödl, A.

AU - Robota, H.

AU - Segner, J.

AU - Vielhaber, W.

AU - Lin, Ming-Chang

AU - Ertl, G.

PY - 1986/4/2

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N2 - The reaction NO2 → NO + Oad at aGe surface was studied by combined molecular beam and laser-induced fluorescence (LIF) techniques. The rotational state distribution of the NO formed is non-Boltzmann, in contrast to NO molecules undergoing trapping/desorption. It is concluded that NO formed by NO2 decomposition is directly released into the gas phase (dissociative desorption) without being intermediately thermally accommodated to the surface.

AB - The reaction NO2 → NO + Oad at aGe surface was studied by combined molecular beam and laser-induced fluorescence (LIF) techniques. The rotational state distribution of the NO formed is non-Boltzmann, in contrast to NO molecules undergoing trapping/desorption. It is concluded that NO formed by NO2 decomposition is directly released into the gas phase (dissociative desorption) without being intermediately thermally accommodated to the surface.

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Reaction dynamics of NO2 decomposition on Ge: An example of dissociative desorption

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Reaction dynamics of NO₂ decomposition on Ge: An example of dissociative desorption