Manipulation of interfacial charge dynamics for metal-organic frameworks toward advanced photocatalytic applications

Chien Yi Wang, Huai En Chang, Cheng Yu Wang*, Tomoyuki Kurioka*, Chun Yi Chen, Tso Fu Mark Chang, Masato Sone, Yung Jung Hsu*

*此作品的通信作者

研究成果: Review article同行評審

摘要

Compared to other known materials, metal-organic frameworks (MOFs) have the highest surface area and the lowest densities; as a result, MOFs are advantageous in numerous technological applications, especially in the area of photocatalysis. Photocatalysis shows tantalizing potential to fulfill global energy demands, reduce greenhouse effects, and resolve environmental contamination problems. To exploit highly active photocatalysts, it is important to determine the fate of photoexcited charge carriers and identify the most decisive charge transfer pathway. Methods to modulate charge dynamics and manipulate carrier behaviors may pave a new avenue for the intelligent design of MOF-based photocatalysts for widespread applications. By summarizing the recent developments in the modulation of interfacial charge dynamics for MOF-based photocatalysts, this minireview can deliver inspiring insights to help researchers harness the merits of MOFs and create versatile photocatalytic systems.

原文English
頁(從 - 到)1039-1058
頁數20
期刊Nanoscale Advances
6
發行號4
DOIs
出版狀態Published - 16 11月 2023

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