Isomers of Ge2N2: Production and infrared absorption of GeNNGe in solid N2

Mohammed Bahou; K. Sankaran; Yu Jong Wu; Yuan-Pern Lee; David Rayner; Benoit Simard

doi:10.1063/1.1569907

Isomers of Ge₂N₂: Production and infrared absorption of GeNNGe in solid N₂

Mohammed Bahou, K. Sankaran, Yu Jong Wu, Yuan-Pern Lee^*, David Rayner, Benoit Simard

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摘要

Laser-ablated Ge reacts with N₂ to form a new species that absorbs near 887.9 cm^-1. Based on observed and calculated vibrational wave numbers and Ge- and N-isotopic shifts, the carrier of observed feature to be linear GeNNGe. Experimental observations that the N-N bond remains intact and that the concentration of linear GeNNGe became enhanced at an increased temperature of deposition and after annealing are consistent with this mechanism.

原文	English
頁（從 - 到）	9710-9718
頁數	9
期刊	Journal of Chemical Physics
卷	118
發行號	21
DOIs	https://doi.org/10.1063/1.1569907
出版狀態	Published - 1 6月 2003

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10.1063/1.1569907

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abstract = "Laser-ablated Ge reacts with N2 to form a new species that absorbs near 887.9 cm-1. Based on observed and calculated vibrational wave numbers and Ge- and N-isotopic shifts, the carrier of observed feature to be linear GeNNGe. Experimental observations that the N-N bond remains intact and that the concentration of linear GeNNGe became enhanced at an increased temperature of deposition and after annealing are consistent with this mechanism.",

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T2 - Production and infrared absorption of GeNNGe in solid N2

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AU - Sankaran, K.

AU - Wu, Yu Jong

AU - Lee, Yuan-Pern

AU - Rayner, David

AU - Simard, Benoit

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N2 - Laser-ablated Ge reacts with N2 to form a new species that absorbs near 887.9 cm-1. Based on observed and calculated vibrational wave numbers and Ge- and N-isotopic shifts, the carrier of observed feature to be linear GeNNGe. Experimental observations that the N-N bond remains intact and that the concentration of linear GeNNGe became enhanced at an increased temperature of deposition and after annealing are consistent with this mechanism.

AB - Laser-ablated Ge reacts with N2 to form a new species that absorbs near 887.9 cm-1. Based on observed and calculated vibrational wave numbers and Ge- and N-isotopic shifts, the carrier of observed feature to be linear GeNNGe. Experimental observations that the N-N bond remains intact and that the concentration of linear GeNNGe became enhanced at an increased temperature of deposition and after annealing are consistent with this mechanism.

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ER -

Isomers of Ge2N2: Production and infrared absorption of GeNNGe in solid N2

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Isomers of Ge₂N₂: Production and infrared absorption of GeNNGe in solid N₂