TY - JOUR
T1 - Graphene and Beyond
T2 - Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices
AU - Lei, Yu
AU - Zhang, Tianyi
AU - Lin, Yu Chuan
AU - Granzier-Nakajima, Tomotaroh
AU - Bepete, George
AU - Kowalczyk, Dorota A.
AU - Lin, Zhong
AU - Zhou, Da
AU - Schranghamer, Thomas F.
AU - Dodda, Akhil
AU - Sebastian, Amritanand
AU - Chen, Yifeng
AU - Liu, Yuanyue
AU - Pourtois, Geoffrey
AU - Kempa, Thomas J.
AU - Schuler, Bruno
AU - Edmonds, Mark T.
AU - Quek, Su Ying
AU - Wurstbauer, Ursula
AU - Wu, Stephen M.
AU - Glavin, Nicholas R.
AU - Das, Saptarshi
AU - Dash, Saroj Prasad
AU - Redwing, Joan M.
AU - Robinson, Joshua A.
AU - Terrones, Mauricio
N1 - Publisher Copyright:
© 2022 American Chemical Society.
PY - 2022/12/21
Y1 - 2022/12/21
N2 - Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moiré pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moiré engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.
AB - Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moiré pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moiré engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.
KW - 2D Materials
KW - Artificial Intelligence
KW - Defect Engineering
KW - Excitonic Properties
KW - Magnetic and Topological Properties
KW - Moiré Engineering
KW - Strain Engineering
KW - Theory-Guided Synthesis
UR - https://www.scopus.com/pages/publications/85139295630
U2 - 10.1021/acsnanoscienceau.2c00017
DO - 10.1021/acsnanoscienceau.2c00017
M3 - Review article
AN - SCOPUS:85139295630
SN - 2694-2496
VL - 2
SP - 450
EP - 485
JO - ACS Nanoscience Au
JF - ACS Nanoscience Au
IS - 6
ER -