A Bis-Cyclopentadienyl Ligand-Supported Di-Iron Trihydride Motif as a Synthon for Access to Heterobimetallic Trinuclear Complexes

Chung Ching Tseng, Yi Wun Ding, Zhong Yue Chen, Hao Yuan Lan, Han Jung Li, You Song Cheng, Ting Shen Kuo, Pei Lin Chen, Wen Chun Wu, Fong Ku Shi, Tzuhsiung Yang, Hsueh Ju Liu*

*此作品的通信作者

研究成果: Article同行評審

摘要

Herein, we report the synthesis of a flexible bis-cyclopentadienyl ligand L (the doubly deprotonated form of H2L (1,3-bis(2,4-di-tert-butylcyclopentadienyldimethylsilyl)benzene)), demonstrating its ability to stabilize a series of di-iron hydrido complexes. Notably, this ligand facilitates the isolation of an unprecedented anionic cyclopentadienyl ligand-supported di-iron trihydride complex, LFe2(μ-H)3Li(THF) (2), functioning as a synthon for the [Fe2(μ-H)3] core and providing access to heterobimetallic complexes 4-6 with coinage metals.

原文English
頁(從 - 到)11361-11368
頁數8
期刊Inorganic Chemistry
63
發行號24
DOIs
出版狀態Published - 17 6月 2024

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