Abstract
A new control scheme of molecular photo-dissociation with use of the complete reflection phenomenon is proposed and demonstrated numerically in the one- and two-dimensional models. In this scheme, an appropriate vibrational excited state is prepared at first and then by applying the stationary laser field with the laser frequency and two NT type avoided crossings are created between the ground electronic bound state dressed up by one photon energy and the excited dissociative electronic state.
| Original language | English |
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| Pages (from-to) | 6197-6209 |
| Number of pages | 13 |
| Journal | Journal of Chemical Physics |
| Volume | 113 |
| Issue number | 15 |
| DOIs | |
| State | Published - 15 Oct 2000 |