Hybrid Plasmonic Surface Lattice Resonance Perovskite Lasers on Silver Nanoparticle Arrays

Zhen Ting Huang; Chih Wei Yin; Yu Heng Hong; Heng Li; Kuo Bin Hong; Tsung-Sheng Kao; Min Hsiung Shih; Tien-Chang Lu

doi:10.1002/adom.202100299

Hybrid Plasmonic Surface Lattice Resonance Perovskite Lasers on Silver Nanoparticle Arrays

Zhen Ting Huang, Chih Wei Yin, Yu Heng Hong, Heng Li, Kuo Bin Hong, Tsung-Sheng Kao, Min Hsiung Shih, Tien-Chang Lu^*

^*Corresponding author for this work

Department of Photonics

Research output: Contribution to journal › Article › peer-review

13 Scopus citations

Abstract

The hybrid plasmonic surface lattice resonance (SLR) laser constructed by a MAPbBr₃ perovskite thin film on the Ag nanoparticle array is unambiguously demonstrated in this research. The relatively high refractive index of the perovskite thin film provides an excellent coupling between the photonic mode and SLR, leading to a high spontaneous emission coupling factor and a low threshold lasing. Furthermore, a novel spin-coating process applied to grow the MAPbBr₃ perovskite thin film can leave air gaps under the perovskite that provides a large index difference in the periodic array, making the hybrid plasmonic SLR exhibits a high density of state, which is beneficial for laser operation. Via theoretical design and experimental verification, the lasing behaviors of the hybrid plasmonic SLR perovskite laser show excellent characteristics with a fixed polarization. This demonstration facilitates an enhanced lasing performance and realization of the low-cost and low-energy-consumption laser application.

Original language	American English
Article number	2100299
Journal	Advanced Optical Materials
Volume	9
Issue number	17
DOIs	https://doi.org/10.1002/adom.202100299
State	Published - 6 Sep 2021

Keywords

hybrid plasmonic mode
perovskites
strong light–matter interaction
surface lattice resonance

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title = "Hybrid Plasmonic Surface Lattice Resonance Perovskite Lasers on Silver Nanoparticle Arrays",

abstract = "The hybrid plasmonic surface lattice resonance (SLR) laser constructed by a MAPbBr3 perovskite thin film on the Ag nanoparticle array is unambiguously demonstrated in this research. The relatively high refractive index of the perovskite thin film provides an excellent coupling between the photonic mode and SLR, leading to a high spontaneous emission coupling factor and a low threshold lasing. Furthermore, a novel spin-coating process applied to grow the MAPbBr3 perovskite thin film can leave air gaps under the perovskite that provides a large index difference in the periodic array, making the hybrid plasmonic SLR exhibits a high density of state, which is beneficial for laser operation. Via theoretical design and experimental verification, the lasing behaviors of the hybrid plasmonic SLR perovskite laser show excellent characteristics with a fixed polarization. This demonstration facilitates an enhanced lasing performance and realization of the low-cost and low-energy-consumption laser application.",

keywords = "hybrid plasmonic mode, perovskites, strong light–matter interaction, surface lattice resonance",

author = "Huang, {Zhen Ting} and Yin, {Chih Wei} and Hong, {Yu Heng} and Heng Li and Hong, {Kuo Bin} and Tsung-Sheng Kao and Shih, {Min Hsiung} and Tien-Chang Lu",

note = "Funding Information: This work was partially supported by the Research Team of Photonic Technologies and Intelligent Systems at National Chiao Tung University within the framework of the Higher Education Sprout Project by the Ministry of Education (MOE) in Taiwan. This work was financially supported by Minister of Science and Technology (MOST) in Taiwan under Contract Nos. MOST 109‐2124‐M‐009‐005, MOST 109‐2221‐E‐009‐150, MOST 107‐2221‐E‐009‐116‐MY3, and MOST 108‐2112‐M‐001‐044‐MY2. Publisher Copyright: {\textcopyright} 2021 Wiley-VCH GmbH",

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AU - Huang, Zhen Ting

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AU - Hong, Kuo Bin

AU - Kao, Tsung-Sheng

AU - Shih, Min Hsiung

AU - Lu, Tien-Chang

N1 - Funding Information: This work was partially supported by the Research Team of Photonic Technologies and Intelligent Systems at National Chiao Tung University within the framework of the Higher Education Sprout Project by the Ministry of Education (MOE) in Taiwan. This work was financially supported by Minister of Science and Technology (MOST) in Taiwan under Contract Nos. MOST 109‐2124‐M‐009‐005, MOST 109‐2221‐E‐009‐150, MOST 107‐2221‐E‐009‐116‐MY3, and MOST 108‐2112‐M‐001‐044‐MY2. Publisher Copyright: © 2021 Wiley-VCH GmbH

PY - 2021/9/6

Y1 - 2021/9/6

N2 - The hybrid plasmonic surface lattice resonance (SLR) laser constructed by a MAPbBr3 perovskite thin film on the Ag nanoparticle array is unambiguously demonstrated in this research. The relatively high refractive index of the perovskite thin film provides an excellent coupling between the photonic mode and SLR, leading to a high spontaneous emission coupling factor and a low threshold lasing. Furthermore, a novel spin-coating process applied to grow the MAPbBr3 perovskite thin film can leave air gaps under the perovskite that provides a large index difference in the periodic array, making the hybrid plasmonic SLR exhibits a high density of state, which is beneficial for laser operation. Via theoretical design and experimental verification, the lasing behaviors of the hybrid plasmonic SLR perovskite laser show excellent characteristics with a fixed polarization. This demonstration facilitates an enhanced lasing performance and realization of the low-cost and low-energy-consumption laser application.

AB - The hybrid plasmonic surface lattice resonance (SLR) laser constructed by a MAPbBr3 perovskite thin film on the Ag nanoparticle array is unambiguously demonstrated in this research. The relatively high refractive index of the perovskite thin film provides an excellent coupling between the photonic mode and SLR, leading to a high spontaneous emission coupling factor and a low threshold lasing. Furthermore, a novel spin-coating process applied to grow the MAPbBr3 perovskite thin film can leave air gaps under the perovskite that provides a large index difference in the periodic array, making the hybrid plasmonic SLR exhibits a high density of state, which is beneficial for laser operation. Via theoretical design and experimental verification, the lasing behaviors of the hybrid plasmonic SLR perovskite laser show excellent characteristics with a fixed polarization. This demonstration facilitates an enhanced lasing performance and realization of the low-cost and low-energy-consumption laser application.

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KW - perovskites

KW - strong light–matter interaction

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Hybrid Plasmonic Surface Lattice Resonance Perovskite Lasers on Silver Nanoparticle Arrays

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Keywords

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