A new ladder-type benzodi(cyclopentadithiophene)-based donor-acceptor polymer and a modified hole-collecting PEDOT:PSS layer to achieve tandem solar cells with an open-circuit voltage of 1.62 v

Yung Lung Chen; Wei Shun Kao; Che En Tsai; Yu Ying Lai; Yen-Ju Cheng; Chain-Shu Hsu

doi:10.1039/c3cc43756f

A new ladder-type benzodi(cyclopentadithiophene)-based donor-acceptor polymer and a modified hole-collecting PEDOT:PSS layer to achieve tandem solar cells with an open-circuit voltage of 1.62 v

Yung Lung Chen, Wei Shun Kao, Che En Tsai, Yu Ying Lai, Yen-Ju Cheng^*, Chain-Shu Hsu

^*Corresponding author for this work

Department of Applied Chemistry

Research output: Contribution to journal › Article › peer-review

27 Scopus citations

Abstract

We have developed a new ladder-type conjugated polymer PBDCPDT-FBT and a robust interconnecting layer (ICL) integrating a hole-collecting m-PEDOT:PSS layer with an electron-collecting ZnO layer. The inverted device using PBDCPDT-FBT exhibited a high power conversion efficiency (PCE) of 5.76% with a V_oc of 0.81 V, a J_sc of 12.82 mA cm^-2, and a FF of 55.5%. The inverted tandem device incorporating the PBDCPDT-FBT and ICL achieves a V_oc of 1.62 V leading to a PCE of 7.08%.

Original language	English
Pages (from-to)	7702-7704
Number of pages	3
Journal	Chemical Communications
Volume	49
Issue number	70
DOIs	https://doi.org/10.1039/c3cc43756f
State	Published - 11 Sep 2013

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title = "A new ladder-type benzodi(cyclopentadithiophene)-based donor-acceptor polymer and a modified hole-collecting PEDOT:PSS layer to achieve tandem solar cells with an open-circuit voltage of 1.62 v",

abstract = "We have developed a new ladder-type conjugated polymer PBDCPDT-FBT and a robust interconnecting layer (ICL) integrating a hole-collecting m-PEDOT:PSS layer with an electron-collecting ZnO layer. The inverted device using PBDCPDT-FBT exhibited a high power conversion efficiency (PCE) of 5.76% with a Voc of 0.81 V, a Jsc of 12.82 mA cm-2, and a FF of 55.5%. The inverted tandem device incorporating the PBDCPDT-FBT and ICL achieves a Voc of 1.62 V leading to a PCE of 7.08%.",

author = "Chen, {Yung Lung} and Kao, {Wei Shun} and Tsai, {Che En} and Lai, {Yu Ying} and Yen-Ju Cheng and Chain-Shu Hsu",

year = "2013",

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doi = "10.1039/c3cc43756f",

language = "English",

volume = "49",

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journal = "Chemical Communications",

issn = "1359-7345",

publisher = "Royal Society of Chemistry",

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A new ladder-type benzodi(cyclopentadithiophene)-based donor-acceptor polymer and a modified hole-collecting PEDOT:PSS layer to achieve tandem solar cells with an open-circuit voltage of 1.62 v. / Chen, Yung Lung; Kao, Wei Shun; Tsai, Che En et al.
In: Chemical Communications, Vol. 49, No. 70, 11.09.2013, p. 7702-7704.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - A new ladder-type benzodi(cyclopentadithiophene)-based donor-acceptor polymer and a modified hole-collecting PEDOT:PSS layer to achieve tandem solar cells with an open-circuit voltage of 1.62 v

AU - Chen, Yung Lung

AU - Kao, Wei Shun

AU - Tsai, Che En

AU - Lai, Yu Ying

AU - Cheng, Yen-Ju

AU - Hsu, Chain-Shu

PY - 2013/9/11

Y1 - 2013/9/11

N2 - We have developed a new ladder-type conjugated polymer PBDCPDT-FBT and a robust interconnecting layer (ICL) integrating a hole-collecting m-PEDOT:PSS layer with an electron-collecting ZnO layer. The inverted device using PBDCPDT-FBT exhibited a high power conversion efficiency (PCE) of 5.76% with a Voc of 0.81 V, a Jsc of 12.82 mA cm-2, and a FF of 55.5%. The inverted tandem device incorporating the PBDCPDT-FBT and ICL achieves a Voc of 1.62 V leading to a PCE of 7.08%.

AB - We have developed a new ladder-type conjugated polymer PBDCPDT-FBT and a robust interconnecting layer (ICL) integrating a hole-collecting m-PEDOT:PSS layer with an electron-collecting ZnO layer. The inverted device using PBDCPDT-FBT exhibited a high power conversion efficiency (PCE) of 5.76% with a Voc of 0.81 V, a Jsc of 12.82 mA cm-2, and a FF of 55.5%. The inverted tandem device incorporating the PBDCPDT-FBT and ICL achieves a Voc of 1.62 V leading to a PCE of 7.08%.

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U2 - 10.1039/c3cc43756f

DO - 10.1039/c3cc43756f

M3 - Article

C2 - 23877029

AN - SCOPUS:84881449747

SN - 1359-7345

VL - 49

SP - 7702

EP - 7704

JO - Chemical Communications

JF - Chemical Communications

IS - 70

ER -

A new ladder-type benzodi(cyclopentadithiophene)-based donor-acceptor polymer and a modified hole-collecting PEDOT:PSS layer to achieve tandem solar cells with an open-circuit voltage of 1.62 v

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